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RuSr2(Nd,Y,Ce)2Cu2O10-d ruthenocuprates have been studied by neutrondiffraction, magnetotransport and magnetisation measurements and the electronicphase diagram is reported. Separate Ru and Cu spin ordering transitions areobserved, with spontaneous Cu antiferromagnetic order for low hole dopinglevels p, and a distinct, induced-antiferromagnetic Cu spin phase in the 0.02 <p < 0.06 pseudogap region. This ordering gives rise to large negativemagnetoresistances which vary systematically with p in theRuSr2Nd1.8-xY0.2CexCu2O10-d series. A collapse of the magnetoresistance (MR)and magnetisation in the pre-superconducting region may signify the onset ofsuperconducting fluctuations.

Induced antiferromagnetism and large magnetoresistances in RuSr2(Nd,Y,Ce)2Cu2O10-d ruthenocuprates