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We examine environmental effects of surrounding nuclear spins on the electronspin relaxation of the N@C60 molecule (which consists of a nitrogen atom at thecentre of a fullerene cage). Using dilute solutions of N@C60 in regular anddeuterated toluene, we observe and model the effect of translational diffusionof nuclear spins of the solvent molecules on the N@C60 electron spin relaxationtimes. We also study spin relaxation in frozen solutions of N@C60 in CS2, towhich small quantities of a glassing agent, S2Cl2 are added. At lowtemperatures, spin relaxation is caused by spectral diffusion of surroundingnuclear 35Cl and 37Cl spins in the S2Cl2, but nevertheless, at 20 K, T2 timesas long as 0.23 ms are observed.Comment: 7 pages, 6 figure

physical review. b, condensed matter and materials physics

Environmental effects on electron spin relaxation in<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:mi mathvariant="normal">N</mml:mi><mml:mi>@</mml:mi><mml:msub><mml:mi mathvariant="normal">C</mml:mi><mml:mn>60</mml:mn></mml:msub></mml:mrow></mml:math>

Environmental effects on electron spin relaxation inN@C60