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Synchrotron X-ray diffraction patterns were measured and analyzed for apolycrystalline sample of the room-temperature ferromagnet Sr3.12Er0.88Co4O10.5from 300 to 650 K, from which two structural phase transitions were found tooccur successively. The higher-temperature transition at 509 K is driven byordering of the oxygen vacancies, which is closely related to the metallicstate at high temperatures. The lower-temperature transition at 360 K is offirst order, at which the ferromagnetic state suddenly appears with exhibitinga jump in magnetization and resistivity. Based on the refined structure,possible spin and orbital models for the magnetic order are proposed.

Structure-Property Relationship in the Ordered-Perovskite- Related Oxide Sr3.12Er0.88Co4O10.5