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A three-level Lambda system in Tm3+ doped YAG crystal is experimentallyinvestigated in the prospect of quantum information processing. Zeeman effectis used to lift the nuclear spin degeneracy of this ion. In a previous paper[de Seze et al. Phys. Rev. B, 73, 85112 (2006) we measured the gyromagnetictensor components and concluded that adequate magnetic field orientation couldoptimize the optical connection of both ground state sublevels to each one ofthe excited state sublevels, thus generating Lambda systems. Here we report onthe direct measurement of the transition probability ratio along the two legsof the Lambda. Measurement techniques combine frequency selective opticalpumping with optical nutation or photon echo processes

physical review. b, condensed matter and materials physics

Branching ratio measurement of a<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>Λ</mml:mi></mml:math>system in<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="normal">Tm</mml:mi><mml:mrow><mml:mn>3</mml:mn><mml:mo>+</mml:mo></mml:mrow></mml:msup><mml:mo>:</mml:mo><mml:mi>YAG</mml:mi></mml:mrow></mml:math>under a magnetic field

Branching ratio measurement of aΛsystem inTm3+:YAGunder a magnetic field