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A 1/2 magnetization plateau in magnetic fields above 23 T andantiferromagnetic (AF) long-range order (AFLRO) in low fields were found inCu$_2$CdB$_2$O$_6$. Experimental results agree with quantum Monte Carlo resultsfor an expected spin system. There are two kinds of Cu sites [Cu(1) and Cu(2)],which are located adjacent to each other. Unexpectedly, spins on the Cu(1) andCu(2) sites are in a nearly spin-singlet state and form AFLRO, respectively,although interactions between the Cu(1) and Cu(2) spins cannot be ignored.Cu$_2$CdB$_2$O$_6$ is the first material which shows such coexistence in anatomic scale.Comment: 5 pages, 4 figure

physical review b

Coexistence of a nearly spin-singlet state and antiferromagnetic long-range order in quantum spin system<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mi>Cu</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi>CdB</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi mathvariant="normal">O</mml:mi><mml:mn>6</mml:mn></mml:msub></mml:mrow></mml:math>

Coexistence of a nearly spin-singlet state and antiferromagnetic long-range order in quantum spin systemCu2CdB2O6