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Magnetic excitations of the filled skutterudite PrRu4P12 exhibiting ametal-insulator (M-I) transition at TM-I= 63 K were studied by inelasticneutron scattering experiment. The spectra at temperatures much lower than TM-Iare described as well-defined crystal-field excitations. With approaching TM-I,the excitation peaks broaden and shift considerably together with thetemperature variation of the carrier number and the atomic displacement in thetransition. The 4f-electron state evolve from the well localized state in theinsulator phase to the strongly hybridized itinerant state by p-f mixing nearTM-I. The hybridization is responsible for the M-I transition of PrRu4P12.Comment: 5 pages, 6 figures, 1 table. Accepted by Phys. Rev.

physical review. b, condensed matter and materials physics

Evolution of<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:mn>4</mml:mn><mml:mi>f</mml:mi></mml:mrow></mml:math>electron states in the metal-insulator transition of<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:mi mathvariant="normal">Pr</mml:mi><mml:msub><mml:mi mathvariant="normal">Ru</mml:mi><mml:mn>4</mml:mn></mml:msub><mml:msub><mml:mi mathvariant="normal">P</mml:mi><mml:mn>12</mml:mn></mml:msub></mml:mrow…

Evolution of4felectron states in the metal-insulator transition ofPrRu4P12