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Using first principles calculations based on the density functional theory and generalized gradient approximation we show that the ground state of Mn doped ZnO $(10\overline{1}0)$ thin film changes from antiferromagnetic to ferromagnetic when codoped with N. The ferromagnetic coupling between Mn spins arises due to the overlap between N $2p$ and Mn $3d$ electrons in the spin up band, rendering the system half-metallic character.

physical review b

Carrier-mediated ferromagnetism in N codoped (Zn,Mn)O<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:mn>10</mml:mn><mml:mover accent="true"><mml:mn>1</mml:mn><mml:mo stretchy="false">¯</mml:mo></mml:mover><mml:mn>0</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:math>thin films

Carrier-mediated ferromagnetism in N codoped (Zn,Mn)O(101¯0)thin films