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The temperature dependent ac and dc magnetization and heat capacity data ofCa$_3$CoIrO$_6$, a spin-chain compound crystallizing in a K$_4$CdCl$_6$-derivedrhombohedral structure, show the features due to magnetic ordering of afrustrated-type below about 30 K, however without exhibiting the signatures ofthe so-called "partially disordered antiferromagnetic structure" encountered inthe isostructural compounds, Ca$_3$Co$_2$O$_6$ and Ca$_3$CoRhO$_6$. This classof compounds thus provides a variety for probing the consequences of magneticfrustration due to topological reasons in stoichiometric spin-chain materials,presumably arising from subtle differences in the interchain and intrachainmagnetic coupling strengths. This compound presents additional interestingsituations in the sense that, ac susceptibility exhibits a large frequencydependence in the vicinity of 30 K uncharacteristic of conventionalspin-glasses, with this frustrated magnetic state being robust to theapplication of external magnetic fields.Comment: Physical Review (Rapid Communications), in pres

physical review. b, condensed matter

Magnetic frustration in the stoichiometric spin-chain compound<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">Ca</mml:mi></mml:mrow><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">CoIrO</mml:mi></mml:mrow><mml:mrow><mml:mn>6</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>

Magnetic frustration in the stoichiometric spin-chain compoundCa3CoIrO6