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We synthesized hexagonal YMnO3 doped with tetravalent Zr ions and studied the electronic and magnetic properties. Zr substitution creates a mixed Mn3+-Mn2+ system, instead of the conventional Mn3+-Mn4+ of colossal magnetoresistance manganites. The YMnO3 system displays a pronounced asymmetry for electron and hole doping. Hole doping results in a conducting state, whereas electron doping retains the insulating state. This asymmetry is a consequence of the crystal field splitting of the Mn ions in trigonal bipyramidal coordination.

physical review. b, condensed matter

Asymmetry of electron and hole doping in<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">YMnO</mml:mi></mml:mrow><mml:mrow><mml:mn>3</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>

Asymmetry of electron and hole doping inYMnO3