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Angle-resolved photoemission was used to investigate the valence-band structure of the metal overlayer system c(10 x 2)Ag/Cu(001). At 1--2 monolayer coverages, the Ag adlayer exhibited d-band spectral behavior characteristic of two-dimensional dispersion. Evaporation of progressively more Ag onto the substrate produced a series of surfaces which by 3--5 monolayer exposures were converging toward a three-dimensional valence electronic structure characteristic of a bulk, Ag(111)-like system.

Ag/Cu(001): Observation of the development of the electronic structure in metal overlayers from two to three dimensionality