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Amorphous alloys of the tin-iron system have been prepared by the vapor-quenching technique. Bulk magnetic data show typical "spin-glass-like" behavior in the low-temperature susceptibility and in the remanent magnetization for alloys containing less than about 40 at.% of iron. A multicritical magnetic phase diagram with paramagnetic, ferromagnetic, and spin-glass-like phases is proposed. High-field magnetization measured up to 150 kOe strongly suggests that local anisotropy, randomly oriented through the material, might successfully compete with exchange interactions for some of the iron clusters.

physical review. b, condensed matter

Magnetic behavior of<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">Fe</mml:mi></mml:mrow><mml:mrow><mml:mi>x</mml:mi></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant="normal">Sn</mml:mi></mml:mrow><mml:mrow><mml:mn>1</mml:mn><mml:mo>−</mml:mo><mml:mi>x</mml:mi></mml:mrow></mml:msub></mml:mrow></mml:math>amorphous alloys near the critical composition

Magnetic behavior ofFexSn1−xamorphous alloys near the critical composition