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We report the experimental observation of Ising superconductivity in3-dimensional NbSe2 stacked with single-layer MoS2. The angular dependence ofthe upper critical magnetic field and the temperature dependence of the upperparallel critical field confirm the appearance of two-dimensional Isingsuperconductivity in the 3-dimensional NbSe2 with single-layer MoS2 overlay. Weshow that the superconducting phase has strong Ising spin-orbit correlationswhich make the holes spin non-degenerate. Our observation of Isingsuperconductivity in heterostructures of few-layer NbSe2 of thickness ~ 15 nmwith single-layer MoS2 raises the interesting prospect of observing topologicalchiral superconductors with nontrivial Chern numbers in a momentum-spacespin-split fermionic system.

Transition from three- to two-dimensional Ising superconductivity in few-layer NbSe2 by proximity effect from van der Waals heterostacking