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Intermetallic silicide compounds, LaScSi and Y$_5$Si$_3$, known for beinghydrogen (H) storage materials, are drawing attention as candidates forelectrides in which anions are substituted by unbound electrons. It is inferredfrom a muon spin rotation experiment that the local field at the muon site(which is the same site as that for H) in these compounds exhibits a largenegative shift under an external magnetic field, which is mostly independent oftemperature. Such anomalous diamagnetism signals a unique property of electrideelectrons associated with transition metals. Moreover, the diamagnetic shiftdecreases with increasing H content, suggesting that the electride electronsexisting coherently in the hollow interstitial positions are adsorbed by H toform hydride ions (H$^-$)

Anomalous diamagnetism of electride electrons in transition metal silicides