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We perform a comparative study of the KCr3As3 and the K2Cr3As3 quasi 1Dcompounds, and show that the strong interplay between the lattice and the spindegrees of freedom promotes a new collinear ferrimagnetic ground state withinthe chains in presence of intrachain antiferromagnetic couplings. We proposethat the interchain antiferromagnetic coupling in KCr3As3 plays a crucial rolefor the experimentally observed spin-glass phase with low critical temperature.In the same region of the parameter space, we predict K2Cr3As3 to benon-magnetic but on the verge of the magnetism, sustaining interchainferromagnetic spin fluctuations while the intrachain spin fluctuations areantiferromagnetic.

Intra-chain collinear magnetism and inter-chain magnetic phases in Cr3As3-K-based materials