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We propose and demonstrate a quantum control scheme for hybrid quantumregisters that can reduce the operation time, and therefore the effects ofrelaxation, compared to existing implementations. It combines resonantexcitation pulses with periods of free precession under the internalHamiltonian of the qubit system. We use this scheme to implement quantum gateslike controlled-NOT operations on electronic and nuclear spins of thenitrogen-vacancy center in diamond. As a specific application, we transferpopulation between electronic and nuclear spin qubits and use it to measure theRabi oscillations of a nuclear spin in a system with multiple coupled spins.

Pulse sequences for controlled 2- and 3-qubit gates in a hybrid quantum register