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The fragmentation of gas phase endohedral fullerene, Ho3N@C80, was investigated using femtosecond near-infrared (NIR) laser pulses with an ion velocity map imaging (VMI) spectrometer. We observed that Ho abundance associated with carbon cage opening dominates at an intensity of 1.1×10 W/cm. As the intensity increases, the Ho yield associated with multifragmentation of the carbon cage exceeds the prominence of Ho associated with the gentler carbon cage opening. Moreover, the power law dependence of Ho on laser intensity indicates that the transition of the most likely fragmentation mechanisms occurs around 2.0×10 W/cm.

Fragmentation of endohedral fullerene Ho3N@C80 in an intense femtosecond near-infrared laser field