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The rotational and hyperfine spectrum of the $X^1\Sigma^+ \rightarrowB^3\Pi_1$ transition in TlF molecules was measured using laser-inducedfluorescence from both a thermal and a cryogenic molecular beam. Rotational andhyperfine constants for the $B$ state are obtained. The large magnetichyperfine interaction of the Tl nuclear spin leads to significant mixing of thelowest $B$ state rotational levels. Updated, more precise measurements of the$B\rightarrow X$ vibrational branching fractions are also presented. Thecombined rovibrational branching fractions allow for the prediction of thenumber of photons that can be scattered in a given TlF optical cycling scheme.

Hyperfine Structure of the $B^3\Pi_1$ State and Predictions of Optical Cycling Behavior in the $X\rightarrow B$ transition of TlF