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We report on detailed studies of electronic and nuclear spin states in the diamond-nitrogen-vacancy (NV) center under weak transverse magnetic fields. We numerically predict and experimentally verify a previously unobserved NV hyperfine level anticrossing (LAC) occurring at bias fields of tens of gauss—two orders of magnitude lower than previously reported LACs at ∼ 500 and ∼ 1000 G axial magnetic fields. We then discuss how the NV ground-state Hamiltonian can be manipulated in this regime to tailor the NV's sensitivity to environmental factors and to map into the nuclear spin state.United States. Dept. of Defense. Assistant Secretary of Defense for Research & Engineering (Air Force Contract No. FA8721-05-C-0002)United States. Office of Naval Research (N00014-13-1-0316)United States. National Aeronautics and Space Administration ( Office of the Chief Technologist’s Space Technology Research Fellowship

Diamond-nitrogen-vacancy electronic and nuclear spin-state anticrossings under weak transverse magnetic fields