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We investigate the onset of photoionization shakeup induced interatomicCoulombic decay (ICD) in He2 at the He+*(n = 2) threshold by detecting two He+ions in coincidence. We find this threshold to be shifted towards higherenergies compared to the same threshold in the monomer. The shifted onset ofion pairs created by ICD is attributed to a recapture of the thresholdphotoelectron after the emission of the faster ICD electron.

Interatomic-Coulombic-decay-induced recapture of photoelectrons in helium dimers