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We present experimental results on the ionization/dissociation of methane infemtosecond pulses of radiation. Angular and intensity dependent yields ofsingly and doubly charged species were measured using an imaging massspectrometer. The measured data shows that all fragments yields exhibit somedegree of anisotropy as a result of them being preferably ejected parallel tothe polarization direction. Additionally, an anomalous perpendicularfragmentation pattern is found for CH\-(2)\+(2+). We find evidence of multipledissociation mechanisms including statistical decay, field assisteddissociation and Coulomb explosion.

Observation of anisotropic fragmentation in methane subjected to femtosecond radiation