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We apply theoretically open-loop quantum optimal control techniques toprovide methods for the verification of various quantum coherent transportmechanisms in natural and artificial light-harvesting complexes under realisticexperimental constraints. We demonstrate that optimally shaped laser pulsesallow to faithfully prepare the photosystem in specified initial states (suchas localized excitation or coherent superposition, i.e. propagating andnon-propagating states) and to probe efficiently the dynamics. These resultsprovide a path towards the discrimination of the different transport pathwaysand to the characterization of environmental properties, enhancing ourunderstanding of the role that coherent processes may play in biologicalcomplexes.

Coherent open-loop optimal control of light-harvesting dynamics