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Cold and ultracold polar molecules with nonzero electronic angular momentumare of great interest for studies in quantum chemistry and control,investigations of novel quantum systems, and precision measurement. However, inmixed electric and magnetic fields, these molecules are generically subject toa large set of avoided crossings among their Zeeman sublevels; in magnetictraps, these crossings lead to distorted potentials and trap loss from electricbias fields. We have characterized these crossings in OH bymicrowave-transferring trapped OH molecules from the upper |f; M = +3/2> paritystate to the lower |e; +3/2> state and observing their trap dynamics under anapplied electric bias field. Our observations are very well described by asimple Landau-Zener model, yielding insight to the rich spectra and dynamics ofpolar radicals in mixed external fields.

Microwave state transfer and adiabatic dynamics of magnetically trapped polar molecules