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The photodetachment dynamics of the atomic oxygen anion O{sup -} has been investigated at 266 nm (4.67 eV) by photoelectron detection in a crossed-beam experiment using a magnetic-bottle electron spectrometer. Taking explicit advantage of the Doppler shift imposed by the moving ion beam on the photoelectron energies, we report both the final-state branching ratio and photoelectron angular distributions. After photoabsorption at 266 nm, the formed electron-oxygen scattering state disintegrates, forming either the excited {sup 1}D or the ground {sup 3}P state of oxygen with a partition of {sup 1}D:{sup 3}P=0.32 {+-} 0.06. The detachment leading to the production of O({sup 3}P) shows an angular distribution of photoelectrons characterized by {beta}{sub P}=0.00 {+-} 0.10 mimicking a pure s-wave detachment, while the detachment into excited O({sup 1}D) occurs with {beta}{sub D}=-0.90{+-}0.10, giving direct evidence of interference between the outgoing s and d waves.

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Photoelectron spectroscopy of<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="normal">O</mml:mi><mml:mrow><mml:mo>−</mml:mo></mml:mrow></mml:msup></mml:mrow></mml:math>at 266 nm: Ratio of ground- and excited-state atomic oxygen production and channel-resolved photoelectron anisotropy parameters

Photoelectron spectroscopy ofO−at 266 nm: Ratio of ground- and excited-state atomic oxygen production and channel-resolved photoelectron anisotropy parameters