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Photoelectron angular distributions from fixed-in-space H{sub 2} molecules exposed to ultrashort xuv laser pulses have been evaluated. The theoretical method is based on the solution of the time-dependent Schroedinger equation in a basis of stationary states that include all electronic and vibrational degrees of freedom. Asymmetric angular distributions are observed as a consequence of the delayed ionization from the H{sub 2} doubly excited states, which induces interferences between gerade and ungerade ionization channels. The analysis of this asymmetry as a function of pulse duration can provide an estimate of the corresponding autoionization widths.

physical review a

Asymmetric electron angular distributions in resonant dissociative photoionization of<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mtext>H</mml:mtext><mml:mn>2</mml:mn></mml:msub></mml:mrow></mml:math>with ultrashort xuv pulses

Asymmetric electron angular distributions in resonant dissociative photoionization ofH2with ultrashort xuv pulses