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We propose a new method for the production of ultracold molecular ions. Thismethod utilizes sympathetic cooling due to the strong collisions betweenappropriately chosen molecular ions and laser-cooled neutral atoms to realizeultracold, internal ground-state molecular ions. In contrast to otherexperiments producing cold molecular ions, our proposed method efficientlycools both the internal and external molecular ion degrees of freedom. Theavailability of an ultracold, absolute ground-state sample of molecular ionswould have broad impact to fields as diverse as quantum chemistry,astrophysics, and fundamental physics; and may lead to the development of arobust, scalable quantum computer.

A new method for producing ultracold molecular ions