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Through solution of the multielectron, semi-relativistic, time-dependentSchr\"{o}dinger equation, we show that angular streaking produces stronglyspin-polarized electrons in a noble gas. The degree of spin polarizationincreases with the Keldysh parameter, so that angular streaking -- ordinarilyapplied to investigate tunneling -- may be repurposed to generate stronglyspin-polarized electron bunches. Additionally, we explore modifications of theangular streaking scheme that also enhance spin polarization.

Enhancing spin polarization using ultrafast angular streaking