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Carbon nanotubes (CNTs) make an ideal one-dimensional (1D) material platformfor the exploration of exotic physical phenomena under extremely strong quantumconfinement. The 1D character of electrons, phonons and excitons in individualCNTs features extraordinary electronic, thermal and optical properties. Sincethe first discovery, they have been continuing to attract interest in variousdisciplines, including chemistry, materials science, physics, and engineering.However, the macroscopic manifestation of such properties is still limited,despite significant efforts for decades. Recently, a controlled vacuumfiltration method has been developed for the preparation of wafer-scale filmsof crystalline chirality-enriched CNTs, and such films immediately enableexciting new fundamental studies and applications. In this review, we willfirst discuss the controlled vacuum filtration technique, and then summarizerecent discoveries in optical spectroscopy studies and optoelectronic deviceapplications using films prepared by this technique.

Science and applications of wafer-scale crystalline carbon nanotube films prepared through controlled vacuum filtration