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Light-induced coherent control of the photoelectron angular distribution (PAD) in neon was recently achieved using the Free-Electron Laser (FEL) at FERMI [1]. This experimental tour de force promises a rich field of possibilities in the control of matter and has prompted new research in this exciting field. In order to gain a better understanding of these processes, we investigated two-pathway interferences in the ionization of neon induced by the fundamental and second harmonic of a femtosecond XUV pulse, i.e., the ω+2ω process. We consider the cases for which either (2p3s)P1 [2] or (2p4s)P1 are chosen as intermediate states to enhance the twophoton ionization probability. Douguet et al.: Photoelectron angular distribution in twoathway ionization of ne n with femtosecond XUV pulses 7

Coherent control of the photoelectron angular distribution in photoionization of neon