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We have studied low-temperature magnetic properties as well ashigh-temperature lithium ion diffusion in the battery cathode materialsLixNi1/3Co1/3Mn1/3O2 by the use of muon spin rotation/relaxation. Our datareveal that the samples enter into a 2D spin-glass state below TSG=12 K. Wefurther show that lithium diffusion channels become active for T>Tdiff=125 Kwhere the Li-ion hopping-rate [nu(T)] starts to increase exponentially.Further, nu(T) is found to fit very well to an Arrhenius type equation and theactivation energy for the diffusion process is extracted as Ea=100 meV.

Lithium Diffusion & Magnetism in Battery Cathode Material LixNi1/3Co1/3Mn1/3O2