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Re-evaluated parameters for the square-well potential model forphotoionization of endo-fullerenes are proposed and employed to reveal thespectacular modifications in the Xe 4d photoionization giant resonance alongthe path from Xe@C60 to Xe@C240 to multi-walled Xe@C60@C240.

Xe 4d photoionization in Xe@C60, Xe@C240, and Xe@C60@C240