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A finite-time fluctuation theorem for the diffusion-influenced surfacereaction A <=> B is investigated for spherical and Janus catalytic particles.The finite-time rates and thermodynamic force are analytically calculated bysolving diffusion equations with the special boundary conditions of thefinite-time fluctuation theorem. Theory is compared with numerical simulationscarried out with two different methods: a random walk algorithm andmultiparticle collision dynamics.

Finite-time fluctuation theorem for diffusion-influenced surface reactions on spherical and Janus catalytic particles