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We have trapped BaF molecules in neon ice, and used laser-inducedfluorescence spectroscopy to map out optical transitions in the trappedmolecules. Our measurements show that the neon lattice does not significantlyperturb certain optical transitions in the trapped molecules. We used one ofthese transitions to polarize the electron spins, detect spin flips and measurehyperfine transitions in the trapped molecules, entirely using lasers. Thisdemonstration with heavy polar molecules opens up new opportunities forprecision measurements of beyond-standard-model physics.

BaF molecules in neon ice: trapping, spectroscopy and optical control of electron spins