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We map out the charge-spin density profile of magneto-electric La2/3Sr1/3MnO3 (LSMO)–BiFeO3 (BFO) heterostructure using soft x-ray resonant magnetic reflectivity. We show that the spatial extent of interface orbitals can extend over a few lattice periods even for an atomically sharp interface. While LSMO magnetization is depleted at the interface, BFO does develop a weak magnetic moment mostly near the interface, probably due to a proximity-induced charge-transfer process. Our study reveals that simultaneous control of electronic and magnetic interfaces is essential in realizing the potential of oxide devices.

new journal of physics

Altered magnetism and new electronic length scales in magneto-electric La2/3Sr1/3MnO3–BiFeO3heterointerface