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EuTiO3 (ETO) has recently experienced an enormous revival of interest becauseof its possible multiferroic properties which are currently in the focus ofresearch. Unfortunately ETO is an unlikely candidate for enlargedmultifunctionality since the mode softening - typical for ferroelectrics -remains incomplete, and the antiferromagnetic properties appear at 5.5K only.However, a strong coupling between lattice and Eu spins exists and leads to theappearance of a magnon-phonon-hybrid mode at elevated temperatures as evidencedby electron paramagnetic resonance (EPR), muon spin rotation ({\mu}SR)experiments and model predictions based on a coupled spin-polarizabilityHamiltonian. This novel finding supports the notion of strongmagneto-dielectric (MD) effects being realized in ETO and opens new strategiesin material design and technological applications.

Hybrid paramagnon phonon modes at elevated temperatures in EuTiO3