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By generating broadband high-harmonic pulses from neon and compensating for attosecond chirp by the material dispersion of argon, the generation of near transform-limited 63 as pulses was achieved. The spectral phase analysis showed that, without proper compensation, the attosecond chirp of the broadband harmonics caused splitting of attosecond high-harmonic pulses in addition to pulse broadening. Although it was attained only within a limited spectral range, the attosecond chirp compensation was successful in bringing out pulse compression over broad harmonics, which signifies the effectiveness of the attosecond chirp compensation by material dispersion.

Attosecond chirp compensation over broadband high-order harmonics to generate near transform-limited 63 as pulses