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The electronic structure modifications of WSe2 upon NO2-adsorption at roomand low temperatures were studied by means of photoelectron spectroscopy. Wefound only moderate changes in the electronic structure, which are manifestedas an upward shift of the WSe2-related bands to the smaller binding energies.The observed effects are modelled within the density functional theoryapproach, where a weak adsorption energy of gas molecules on the surface ofWSe2 was deduced. The obtained experimental data are explained as a valencebands polarisation effect, which causes their energy shift depending on theadsorption geometry and the formed dipole moment.

Adsorption of NO2 on WSe2: DFT and photoelectron spectroscopy studies