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The crystal structures and the physical (magnetic, electrical transport andthermodynamic) properties of the ternary compounds CeRhSi2 and Ce2Rh3Si5(orthorhombic CeNiSi2- and U2Co3Si5-type structures, respectively) were studiedin wide ranges of temperature and magnetic field strength. The results revealedthat both materials are valence fluctuating systems, in line with previousliterature reports. Direct evidence for valence fluctuations was obtained bymeans of Ce LIII-edge x-ray absorption spectroscopy and Ce 3d core-level x-rayphotoelectron spectroscopy. The experimental data were confronted with theresults of ab initio calculations of the electronic band structures in bothcompounds.

Magnetic properties and electronic structures of intermediate valence systems CeRhSi2 and Ce2Rh3Si5