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The magnetic properties of Na(2)CuP(2)O(7) were investigated by means of (31)P nuclear magnetic resonance (NMR), magnetic susceptibility, and heat capacity measurements. We report the (31)P NMR shift, the spin-lattice [Formula: see text], and spin-spin (1/T(2)) relaxation rate data as a function of temperature T. The temperature dependence of the NMR shift K(T) is well described by the S = 1/2 square lattice Heisenberg antiferromagnetic model with an intraplanar exchange of [Formula: see text] K and a hyperfine coupling A = 3533 ± 185 Oe /μ(B). The (31)P NMR spectrum was found to broaden abruptly below T∼10 K, signifying some kind of transition. However, no anomaly was noticed in the bulk susceptibility data down to 1.8 K. The heat capacity appears to have a weak maximum around 10 K. With decrease in temperature, the spin-lattice relaxation rate 1/T(1) decreases monotonically and appears to agree well with the high temperature series expansion expression for a S = 1/2 2D square lattice.

31P NMR study of Na2CuP2O7: an S = 1/2 two dimensional Heisenberg antiferromagnetic system

³¹P NMR study of Na₂CuP₂O₇: an S = 1/2 two dimensional Heisenberg antiferromagnetic system