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Considering the photoionization of Ar@C60 and Kr@C60 endofullerenes, thedecay of C60 innershell excitations through the outershell continuum of theconfined atom via the inter-Coulombic decay (ICD) pathway is detailed.Excitations to atom-C60 hybrid states demonstrate coherence between ICD andelectron-transfer mediated decay (ETMD). This should be the dominantabove-threshold decay process for a variety of confined systems, and thestrength of these resonances is such that they should be amenable for study byphotoelectron spectroscopy.

First prediction of inter-Coulombic decay of C60 inner vacancies through the continuum of confined atoms