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We use a simplified self-consistent method to address nonlinear-opticalcascading phenomena, which shows added microscopic cascading contributions inhigh-ordered nonlinear susceptibilities through fifth order. These cascadingterms in the microscopic regime encompass all possible scalar cascadingconfigurations. The imposition of geometric constraints further influences thepredicted cascading contributions and opens up additional design parameters fornonlinear-optical materials. These results are used in approximating theeffective fifth-order susceptibility in thin films of C60 monomers of varyingthickness and concentration. This paper contains the corrections to theoriginal paper that appeared in the Journal of Physics B as reflected in thecontent of the corrigendum that followed.

The Local Field Factor and Microscopic Cascading: A Self-Consistent Method Applied to Confined Systems of Molecules