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An analysis of the magnetocaloric properties of the pure and substituted Fe2Pcompounds is made based on KKR-CPA electronic structure calculations andmagnetisation M(H,T) measurements. The computed electronic densities of statesand magnetic moments are used to calculate both the values of the electronicand magnetic entropies, which fairly agree with the experimental findings. Toenlighten the magnetic properties above Curie temperature, the paramagneticstate behaviours are simulated using the disordered local moments (DLM)concept. The KKR-CPA computations show, that in Fe2P, the Fe magnetic moment ofthe (3f) site disappears in the DLM state, while the moment of the (3g) site isonly little lowered, comparison made with the low temperature ferromagneticstate.

Magnetocaloric properties of Fe_{2-x}T_xP (T = Ru and Rh) from electronic structure calculations and magnetisation measurements