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Gel polymer electrolytes with polyurethane acrylate (PUA) and tetrapropylammonium iodide (TPAI) have been prepared. The maximum conductivity of (4.95 ± 0.02)×10 −5  S cm −1  was obtained after 35 wt.% TPAI is added to PUA (G5 electrolyte), dominated by the highest charge carrier mobility ( µ ). The perovskite solar cell (PSC) with G5 electrolyte displayed the highest power conversion efficiency of (0.206 ± 0.014)%, caused by the highest  µ  in electrolyte G5 that accelerates the electron transfer from the counter electrode to the ionized perovskite. This research proves that PUA can be exploited as a host polymer in polymer electrolytes for PSC applications.

Novel polymer electrolyte based polyurethane acrylate for low-cost perovskite solar cells applications