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Herein, a novel conducting polymer poly(2,5-bis(5-(2,3-dihydrothieno[3,4-b][1, 4]dioxin-5-yl)-3-dodecylthiophen-2-yl)thieno[3,2-b]thiophene) has been developed and synthesized via in situ oxidative polymerization using FeCl 3  as the oxidant. This polymer can be proton doped, and the doping process is reversible. The proton-doped film exhibits  p -type conduction, with a Seebeck coefficient of ca. 24 µV/K, and an electrical conductivity of ca. 30 S·cm −1  with a carrier density of 2 × 10 20  cm −3  has been achieved. This work introduces a new approach for designing proton-dopable organic semiconductors: exchanging and modifying the chemical structure to enable precise tuning of the semiconductor’s properties.

Reversible protonic doping of poly(2,5-bis(5-(2,3-dihydrothieno[3,4-b][1, 4]dioxin-5-yl)-3-dodecylthiophen-2-yl)thieno[3,2-b]thiophene)