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Recently, considerable researches are conducted to develop promising polymer electrolytes for Li-ion batteries (LIBs). Herein, we prepared poly(lithium acrylate) (PAALi)-based composite polymer electrolytes (CPEs) containing alumina (Al 2 O 3 ) nanoparticles. The addition of inorganic nanoparticles into the PAALi matrix can not only improve CPE’s ionic conductivity (at 303 K), but also enhance CPE’s mechanical properties due to the nanoparticles acting as cross-linkers between the PAALi chains. We systematically investigated the influences of inorganic nanoparticle types (pure alumina vs. vinyl functionalized alumina) and contents on ionic conduction and mechanical properties of PAALi-based CPEs.

The effect of inorganic nanoparticles on ion conduction in poly(lithium acrylate)-based composite polymer electrolytes for energy storage devices