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Na 3+x [(Zr/Cr) x (Sc/Ti) 2-x (PO 4 ) 3 ] glass-ceramic material compositions containing NASICON-type crystalline phases might be a good candidate as an efficient electrolyte exclusively for Na-ion batteries. All-solid-state Na-ion full cells are designed with the three-layered pellets (NaCo 0.7 (VO) 0.3 PO 4 /Na 3.5 Zr 0.5 Sc 1.5 (PO 4 ) 3  (NZSP) and Na 3.5 Cr 0.5 Ti 1.5 (PO 4 ) 3 ) (NCTP)/Na-metal foil). The electrical conductivity of the NZSPglass-ceramic powder sample achieves to be highest (9.47 × 10 −04  S/cm) due to its lower grain boundary resistance ( Rgb ) as observed in SEM images and also exhibits best electrochemical stability against conductivity when the samples kept in ambient air for 60 d. The charge/discharge capacities for the initial cycle are 75/69 and 60/53 mAhg −1  to both NZSP and NCTP of two full cells, respectively. However, discharge capacities are boosted up for both these cells without much loss in coulombic efficiency even after 10 cycles.

Glass-Ceramic Na 3+x [(Zr/Cr) x (Sc/Ti) 2-x (PO 4 ) 3 Electrolyte Materials for Na-Ion Full-Cell Application