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Lead-free (1- x )BiFeO 3 - x BaTiO 3  ceramics (abbreviated as BF- x BT), in a composition range of 0.23 ≤  x  ≤ 0.33 mol%, were prepared by the conventional solid-state reaction method. The effect of  x  content on phase structure, microstructure, magnetic and electrical properties of BF- x BT ceramics is also investigated. With the incorporation of  x  content, the coexistence of rhombohedral and tetragonal phases was observed. Field emission scanning electron microscope (FESEM) micrographs revealed that the average grain size of BF- x BT ceramics first decreased and then increased with adding  x  content. The fracture surface of samples showed a mode of inter-granular fracture and intra-granular fracture. The ferroelectric properties were enhanced by adding  x  ≥ 0.29 mol% in the BF- x BT system. The dielectric and magnetic properties were improved with a maximum value are  ε r= 888,711,  Mmax  = 0.40 emu/g,  Mr  = 0.17 emu/g, and  Hc  = 3.7 kOe at  x  = 0.25 mol%

Multiferroic Properties of (1- x )BiFeO 3 - x BaTiO 3 Lead-Free Ceramics