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Sulfur-containing functional groups, among various coordinating functions, have recently attracted attention as useful directing groups for the direct catalytic C-H transformation of aromatic and heteroaromatic compounds. Herein we briefly summarize our recent work on the site-selective substitution on indole and naphthalene skeletons using thioether directing groups under either Cp*Rh(III) or Cp*Ir(III) catalysis. The thioether groups can readily be removed and transformed to other functional groups. The reactions developed appear to be of importance in pharmaceutical and materials chemistry.

Utilization of sulfur function in directed catalytic C-H transformation: site-selective substitution on indole and naphthalene skeletons