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Sterically protected low-coordinate organophosphorus compounds such as diphosphenes, phosphaalkenes, 1,3-diphosphaallenes, 1-phosphaallenes, phosphaalkynes, and 3,4-diphosphinidenecyclobutenes are described, which are stabilized with an extremely bulky 2,4,6-tri- t -butylphenyl (Mes*) group. The structures, physical and chemical properties are highly interesting, because they are unusual phosphorus compounds.

Low coordinate phosphorus compounds for 40 years in memory of the late professor François Mathey, Ecole Polytechnique