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Herein, we synthesized biological magnetic glycoluril tetrakis(methylene phosphorous acid) as a new heterogeneous nano-catalyst. The magnetic nano-catalyst Fe 3 O 4 @GTMPA was used for the synthesis of diphenyl nicotinonitrile derivatives by multi-component reaction of wide spread aldehydes, acetophenones, ammonium acetate, and 3-(1 H -indol-3-yl)-3-oxopropanenitrile in the solvent-free conditions at 110 °C. The final step of reaction mechanism was preceded  via  a cooperative vinylogous anomeric-based oxidation (CVABO) as green and convenient approach.

polycyclic aromatic compounds

Synthesis and Application of Novel Magnetic Glycoluril Tetrakis(Methylene Phosphorous Acid) as a Nano Biological Catalyst for the Preparation of Nicotinonitriles  via  a Cooperative Vinylogous Anomeric-Based Oxidation