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Polycyclic aromatic hydrocarbons (PAHs) as polar organic pollutants, their potential harm to the environment has caused widespread concern. This study describes a simple method to prepare modified aerobic granular sludge (AGS) by hydroxypropyl-β-cyclodextrin (HP-β-CD). Using HP-β-CD modified AGS as the adsorbent, the removal of specific PAHs: Fluoranthene (Fla) reached 95% comparing to 80% of the unmodified AGS. The removal of Fla was related to initial concentration, temperature and ion concentration (Na + , Mg 2+ ). The removal efficiency of Fla reached 96.27%, 94.26% and 93.69%, when initial concentration of Fla was 10, 15 and 20 μmol/L. At temperatures of 15°C, 30°C and 45°C, the removal efficiency of Fla (15 μmol/L) gradually improved from 87.20% to 94.84% and 95.73%. The presence of Na +  and Mg 2+  ions led to the deterioration of PAHs removal. With the increase of Na +  and Mg 2+  concentrations, the removal efficiency of modified AGS on PAHs decreased by 3.9% and 6.5%, respectively .  These findings indicate the potential application of cyclodextrins as the active sites of a complex modified polymer network for PAHs wastewater treatment.

Hydroxypropyl-β-cyclodextrin improves the removal of polycyclic aromatic hydrocarbons by aerobic granular sludge